Source code for ase.io.espresso

"""Reads Quantum ESPRESSO files.

Read multiple structures and results from pw.x output files. Read
structures from pw.x input files.

Built for PWSCF v.5.3.0 but should work with earlier and later versions.
Can deal with most major functionality, but might fail with ibrav =/= 0
or crystal_sg positions.

Units are converted using CODATA 2006, as used internally by Quantum
ESPRESSO.
"""

import os
import operator as op
import re
import warnings
from collections import OrderedDict
from os import path

import numpy as np

from ase.atoms import Atoms
from ase.calculators.singlepoint import (SinglePointDFTCalculator,
                                         SinglePointKPoint)
from ase.calculators.calculator import kpts2ndarray, kpts2sizeandoffsets
from ase.dft.kpoints import kpoint_convert
from ase.constraints import FixAtoms, FixCartesian
from ase.data import chemical_symbols, atomic_numbers
from ase.units import create_units
from ase.utils import iofunction


# Quantum ESPRESSO uses CODATA 2006 internally
units = create_units('2006')

# Section identifiers
_PW_START = 'Program PWSCF'
_PW_END = 'End of self-consistent calculation'
_PW_CELL = 'CELL_PARAMETERS'
_PW_POS = 'ATOMIC_POSITIONS'
_PW_MAGMOM = 'Magnetic moment per site'
_PW_FORCE = 'Forces acting on atoms'
_PW_TOTEN = '!    total energy'
_PW_STRESS = 'total   stress'
_PW_FERMI = 'the Fermi energy is'
_PW_HIGHEST_OCCUPIED = 'highest occupied level'
_PW_HIGHEST_OCCUPIED_LOWEST_FREE = 'highest occupied, lowest unoccupied level'
_PW_KPTS = 'number of k points='
_PW_BANDS = _PW_END
_PW_BANDSTRUCTURE = 'End of band structure calculation'


class Namelist(OrderedDict):
    """Case insensitive dict that emulates Fortran Namelists."""
    def __contains__(self, key):
        return super(Namelist, self).__contains__(key.lower())

    def __delitem__(self, key):
        return super(Namelist, self).__delitem__(key.lower())

    def __getitem__(self, key):
        return super(Namelist, self).__getitem__(key.lower())

    def __setitem__(self, key, value):
        super(Namelist, self).__setitem__(key.lower(), value)

    def get(self, key, default=None):
        return super(Namelist, self).get(key.lower(), default)


[docs]@iofunction('rU') def read_espresso_out(fileobj, index=-1, results_required=True): """Reads Quantum ESPRESSO output files. The atomistic configurations as well as results (energy, force, stress, magnetic moments) of the calculation are read for all configurations within the output file. Will probably raise errors for broken or incomplete files. Parameters ---------- fileobj : file|str A file like object or filename index : slice The index of configurations to extract. results_required : bool If True, atomistic configurations that do not have any associated results will not be included. This prevents double printed configurations and incomplete calculations from being returned as the final configuration with no results data. Yields ------ structure : Atoms The next structure from the index slice. The Atoms has a SinglePointCalculator attached with any results parsed from the file. """ # work with a copy in memory for faster random access pwo_lines = fileobj.readlines() # TODO: index -1 special case? # Index all the interesting points indexes = { _PW_START: [], _PW_END: [], _PW_CELL: [], _PW_POS: [], _PW_MAGMOM: [], _PW_FORCE: [], _PW_TOTEN: [], _PW_STRESS: [], _PW_FERMI: [], _PW_HIGHEST_OCCUPIED: [], _PW_HIGHEST_OCCUPIED_LOWEST_FREE: [], _PW_KPTS: [], _PW_BANDS: [], _PW_BANDSTRUCTURE: [], } for idx, line in enumerate(pwo_lines): for identifier in indexes: if identifier in line: indexes[identifier].append(idx) # Configurations are either at the start, or defined in ATOMIC_POSITIONS # in a subsequent step. Can deal with concatenated output files. all_config_indexes = sorted(indexes[_PW_START] + indexes[_PW_POS]) # Slice only requested indexes # setting results_required argument stops configuration-only # structures from being returned. This ensures the [-1] structure # is one that has results. Two cases: # - SCF of last configuration is not converged, job terminated # abnormally. # - 'relax' and 'vc-relax' re-prints the final configuration but # only 'vc-relax' recalculates. if results_required: results_indexes = sorted(indexes[_PW_TOTEN] + indexes[_PW_FORCE] + indexes[_PW_STRESS] + indexes[_PW_MAGMOM] + indexes[_PW_BANDS] + indexes[_PW_BANDSTRUCTURE]) # Prune to only configurations with results data before the next # configuration results_config_indexes = [] for config_index, config_index_next in zip( all_config_indexes, all_config_indexes[1:] + [len(pwo_lines)]): if any([config_index < results_index < config_index_next for results_index in results_indexes]): results_config_indexes.append(config_index) # slice from the subset image_indexes = results_config_indexes[index] else: image_indexes = all_config_indexes[index] # Extract initialisation information each time PWSCF starts # to add to subsequent configurations. Use None so slices know # when to fill in the blanks. pwscf_start_info = dict((idx, None) for idx in indexes[_PW_START]) for image_index in image_indexes: # Find the nearest calculation start to parse info. Needed in, # for example, relaxation where cell is only printed at the # start. if image_index in indexes[_PW_START]: prev_start_index = image_index else: # The greatest start index before this structure prev_start_index = [idx for idx in indexes[_PW_START] if idx < image_index][-1] # add structure to reference if not there if pwscf_start_info[prev_start_index] is None: pwscf_start_info[prev_start_index] = parse_pwo_start( pwo_lines, prev_start_index) # Get the bounds for information for this structure. Any associated # values will be between the image_index and the following one, # EXCEPT for cell, which will be 4 lines before if it exists. for next_index in all_config_indexes: if next_index > image_index: break else: # right to the end of the file next_index = len(pwo_lines) # Get the structure # Use this for any missing data prev_structure = pwscf_start_info[prev_start_index]['atoms'] if image_index in indexes[_PW_START]: structure = prev_structure.copy() # parsed from start info else: if _PW_CELL in pwo_lines[image_index - 5]: # CELL_PARAMETERS would be just before positions if present cell, cell_alat = get_cell_parameters( pwo_lines[image_index - 5:image_index]) else: cell = prev_structure.cell cell_alat = pwscf_start_info[prev_start_index]['alat'] # give at least enough lines to parse the positions # should be same format as input card n_atoms = len(prev_structure) positions_card = get_atomic_positions( pwo_lines[image_index:image_index + n_atoms + 1], n_atoms=n_atoms, cell=cell, alat=cell_alat) # convert to Atoms object symbols = [label_to_symbol(position[0]) for position in positions_card] positions = [position[1] for position in positions_card] structure = Atoms(symbols=symbols, positions=positions, cell=cell, pbc=True) # Extract calculation results # Energy energy = None for energy_index in indexes[_PW_TOTEN]: if image_index < energy_index < next_index: energy = float( pwo_lines[energy_index].split()[-2]) * units['Ry'] # Forces forces = None for force_index in indexes[_PW_FORCE]: if image_index < force_index < next_index: # Before QE 5.3 'negative rho' added 2 lines before forces # Use exact lines to stop before 'non-local' forces # in high verbosity if not pwo_lines[force_index + 2].strip(): force_index += 4 else: force_index += 2 # assume contiguous forces = [ [float(x) for x in force_line.split()[-3:]] for force_line in pwo_lines[force_index:force_index + len(structure)]] forces = np.array(forces) * units['Ry'] / units['Bohr'] # Stress stress = None for stress_index in indexes[_PW_STRESS]: if image_index < stress_index < next_index: sxx, sxy, sxz = pwo_lines[stress_index + 1].split()[:3] _, syy, syz = pwo_lines[stress_index + 2].split()[:3] _, _, szz = pwo_lines[stress_index + 3].split()[:3] stress = np.array([sxx, syy, szz, syz, sxz, sxy], dtype=float) # sign convention is opposite of ase stress *= -1 * units['Ry'] / (units['Bohr'] ** 3) # Magmoms magmoms = None for magmoms_index in indexes[_PW_MAGMOM]: if image_index < magmoms_index < next_index: magmoms = [ float(mag_line.split()[5]) for mag_line in pwo_lines[magmoms_index + 1: magmoms_index + 1 + len(structure)]] # Fermi level / highest occupied level efermi = None for fermi_index in indexes[_PW_FERMI]: if image_index < fermi_index < next_index: efermi = float(pwo_lines[fermi_index].split()[-2]) if efermi is None: for ho_index in indexes[_PW_HIGHEST_OCCUPIED]: if image_index < ho_index < next_index: efermi = float(pwo_lines[ho_index].split()[-1]) if efermi is None: for holf_index in indexes[_PW_HIGHEST_OCCUPIED_LOWEST_FREE]: if image_index < holf_index < next_index: efermi = float(pwo_lines[holf_index].split()[-2]) # K-points ibzkpts = None weights = None kpoints_warning = "Number of k-points >= 100: " + \ "set verbosity='high' to print them." for kpts_index in indexes[_PW_KPTS]: nkpts = int(pwo_lines[kpts_index].split()[4]) kpts_index += 2 if pwo_lines[kpts_index].strip() == kpoints_warning: continue # QE prints the k-points in units of 2*pi/alat # with alat defined as the length of the first # cell vector cell = structure.get_cell() alat = np.linalg.norm(cell[0]) ibzkpts = [] weights = [] for i in range(nkpts): L = pwo_lines[kpts_index + i].split() weights.append(float(L[-1])) coord = np.array([L[-6], L[-5], L[-4].strip('),')], dtype=float) coord *= 2 * np.pi / alat coord = kpoint_convert(cell, ckpts_kv=coord) ibzkpts.append(coord) ibzkpts = np.array(ibzkpts) weights = np.array(weights) # Bands kpts = None kpoints_warning = "Number of k-points >= 100: " + \ "set verbosity='high' to print the bands." for bands_index in indexes[_PW_BANDS] + indexes[_PW_BANDSTRUCTURE]: if image_index < bands_index < next_index: bands_index += 2 if pwo_lines[bands_index].strip() == kpoints_warning: continue assert ibzkpts is not None spin, bands, eigenvalues = 0, [], [[], []] while True: L = pwo_lines[bands_index].replace('-', ' -').split() if len(L) == 0: if len(bands) > 0: eigenvalues[spin].append(bands) bands = [] elif L == ['occupation', 'numbers']: # Skip the lines with the occupation numbers bands_index += len(eigenvalues[spin][0]) // 8 + 1 elif L[0] == 'k' and L[1].startswith('='): pass elif 'SPIN' in L: if 'DOWN' in L: spin += 1 else: try: bands.extend(map(float, L)) except ValueError: break bands_index += 1 if spin == 1: assert len(eigenvalues[0]) == len(eigenvalues[1]) assert len(eigenvalues[0]) == len(ibzkpts), \ (np.shape(eigenvalues), len(ibzkpts)) kpts = [] for s in range(spin + 1): for w, k, e in zip(weights, ibzkpts, eigenvalues[s]): kpt = SinglePointKPoint(w, s, k, eps_n=e) kpts.append(kpt) # Put everything together # # I have added free_energy. Can and should we distinguish # energy and free_energy? --askhl calc = SinglePointDFTCalculator(structure, energy=energy, free_energy=energy, forces=forces, stress=stress, magmoms=magmoms, efermi=efermi, ibzkpts=ibzkpts) calc.kpts = kpts structure.calc = calc yield structure
def parse_pwo_start(lines, index=0): """Parse Quantum ESPRESSO calculation info from lines, starting from index. Return a dictionary containing extracted information. - `celldm(1)`: lattice parameters (alat) - `cell`: unit cell in Angstrom - `symbols`: element symbols for the structure - `positions`: cartesian coordinates of atoms in Angstrom - `atoms`: an `ase.Atoms` object constructed from the extracted data Parameters ---------- lines : list[str] Contents of PWSCF output file. index : int Line number to begin parsing. Only first calculation will be read. Returns ------- info : dict Dictionary of calculation parameters, including `celldm(1)`, `cell`, `symbols`, `positions`, `atoms`. Raises ------ KeyError If interdependent values cannot be found (especially celldm(1)) an error will be raised as other quantities cannot then be calculated (e.g. cell and positions). """ # TODO: extend with extra DFT info? info = {} for idx, line in enumerate(lines[index:], start=index): if 'celldm(1)' in line: # celldm(1) has more digits than alat!! info['celldm(1)'] = float(line.split()[1]) * units['Bohr'] info['alat'] = info['celldm(1)'] elif 'number of atoms/cell' in line: info['nat'] = int(line.split()[-1]) elif 'number of atomic types' in line: info['ntyp'] = int(line.split()[-1]) elif 'crystal axes:' in line: info['cell'] = info['celldm(1)'] * np.array([ [float(x) for x in lines[idx + 1].split()[3:6]], [float(x) for x in lines[idx + 2].split()[3:6]], [float(x) for x in lines[idx + 3].split()[3:6]]]) elif 'positions (alat units)' in line: info['symbols'], info['positions'] = [], [] for at_line in lines[idx + 1:idx + 1 + info['nat']]: sym, x, y, z = parse_position_line(at_line) info['symbols'].append(label_to_symbol(sym)) info['positions'].append([x * info['celldm(1)'], y * info['celldm(1)'], z * info['celldm(1)']]) # This should be the end of interesting info. # Break here to avoid dealing with large lists of kpoints. # Will need to be extended for DFTCalculator info. break # Make atoms for convenience info['atoms'] = Atoms(symbols=info['symbols'], positions=info['positions'], cell=info['cell'], pbc=True) return info def parse_position_line(line): """Parse a single line from a pw.x output file. The line must contain information about the atomic symbol and the position, e.g. 995 Sb tau( 995) = ( 1.4212023 0.7037863 0.1242640 ) Parameters ---------- line : str Line to be parsed. Returns ------- sym : str Atomic symbol. x : float x-position. y : float y-position. z : float z-position. """ pat = re.compile(r'\s*\d+\s*(\S+)\s*tau\(\s*\d+\)\s*=' r'\s*\(\s*(\S+)\s+(\S+)\s+(\S+)\s*\)') match = pat.match(line) assert match is not None sym, x, y, z = match.group(1, 2, 3, 4) return sym, float(x), float(y), float(z)
[docs]@iofunction('rU') def read_espresso_in(fileobj): """Parse a Quantum ESPRESSO input files, '.in', '.pwi'. ESPRESSO inputs are generally a fortran-namelist format with custom blocks of data. The namelist is parsed as a dict and an atoms object is constructed from the included information. Parameters ---------- fileobj : file | str A file-like object that supports line iteration with the contents of the input file, or a filename. Returns ------- atoms : Atoms Structure defined in the input file. Raises ------ KeyError Raised for missing keys that are required to process the file """ # parse namelist section and extract remaining lines data, card_lines = read_fortran_namelist(fileobj) # get the cell if ibrav=0 if 'system' not in data: raise KeyError('Required section &SYSTEM not found.') elif 'ibrav' not in data['system']: raise KeyError('ibrav is required in &SYSTEM') elif data['system']['ibrav'] == 0: # celldm(1) is in Bohr, A is in angstrom. celldm(1) will be # used even if A is also specified. if 'celldm(1)' in data['system']: alat = data['system']['celldm(1)'] * units['Bohr'] elif 'A' in data['system']: alat = data['system']['A'] else: alat = None cell, cell_alat = get_cell_parameters(card_lines, alat=alat) else: alat, cell = ibrav_to_cell(data['system']) # species_info holds some info for each element species_card = get_atomic_species(card_lines, n_species=data['system']['ntyp']) species_info = {} for ispec, (label, weight, pseudo) in enumerate(species_card): symbol = label_to_symbol(label) valence = get_valence_electrons(symbol, data, pseudo) # starting_magnetization is in fractions of valence electrons magnet_key = "starting_magnetization({0})".format(ispec + 1) magmom = valence * data["system"].get(magnet_key, 0.0) species_info[symbol] = {"weight": weight, "pseudo": pseudo, "valence": valence, "magmom": magmom} positions_card = get_atomic_positions( card_lines, n_atoms=data['system']['nat'], cell=cell, alat=alat) symbols = [label_to_symbol(position[0]) for position in positions_card] positions = [position[1] for position in positions_card] magmoms = [species_info[symbol]["magmom"] for symbol in symbols] # TODO: put more info into the atoms object # e.g magmom, forces. atoms = Atoms(symbols=symbols, positions=positions, cell=cell, pbc=True, magmoms=magmoms) return atoms
def ibrav_to_cell(system): """ Convert a value of ibrav to a cell. Any unspecified lattice dimension is set to 0.0, but will not necessarily raise an error. Also return the lattice parameter. Parameters ---------- system : dict The &SYSTEM section of the input file, containing the 'ibrav' setting, and either celldm(1)..(6) or a, b, c, cosAB, cosAC, cosBC. Returns ------- alat, cell : float, np.array Cell parameter in Angstrom, and The 3x3 array representation of the cell. Raises ------ KeyError Raise an error if any required keys are missing. NotImplementedError Only a limited number of ibrav settings can be parsed. An error is raised if the ibrav interpretation is not implemented. """ if 'celldm(1)' in system and 'a' in system: raise KeyError('do not specify both celldm and a,b,c!') elif 'celldm(1)' in system: # celldm(x) in bohr alat = system['celldm(1)'] * units['Bohr'] b_over_a = system.get('celldm(2)', 0.0) c_over_a = system.get('celldm(3)', 0.0) cosab = system.get('celldm(4)', 0.0) cosac = system.get('celldm(5)', 0.0) cosbc = 0.0 if system['ibrav'] == 14: cosbc = system.get('celldm(4)', 0.0) cosac = system.get('celldm(5)', 0.0) cosab = system.get('celldm(6)', 0.0) elif 'a' in system: # a, b, c, cosAB, cosAC, cosBC in Angstrom alat = system['a'] b_over_a = system.get('b', 0.0) / alat c_over_a = system.get('c', 0.0) / alat cosab = system.get('cosab', 0.0) cosac = system.get('cosac', 0.0) cosbc = system.get('cosbc', 0.0) else: raise KeyError("Missing celldm(1) or a cell parameter.") if system['ibrav'] == 1: cell = np.identity(3) * alat elif system['ibrav'] == 2: cell = np.array([[-1.0, 0.0, 1.0], [0.0, 1.0, 1.0], [-1.0, 1.0, 0.0]]) * (alat / 2) elif system['ibrav'] == 3: cell = np.array([[1.0, 1.0, 1.0], [-1.0, 1.0, 1.0], [-1.0, -1.0, 1.0]]) * (alat / 2) elif system['ibrav'] == -3: cell = np.array([[-1.0, 1.0, 1.0], [1.0, -1.0, 1.0], [1.0, 1.0, -1.0]]) * (alat / 2) elif system['ibrav'] == 4: cell = np.array([[1.0, 0.0, 0.0], [-0.5, 0.5 * 3**0.5, 0.0], [0.0, 0.0, c_over_a]]) * alat elif system['ibrav'] == 5: tx = ((1.0 - cosab) / 2.0)**0.5 ty = ((1.0 - cosab) / 6.0)**0.5 tz = ((1 + 2 * cosab) / 3.0)**0.5 cell = np.array([[tx, -ty, tz], [0, 2 * ty, tz], [-tx, -ty, tz]]) * alat elif system['ibrav'] == -5: ty = ((1.0 - cosab) / 6.0)**0.5 tz = ((1 + 2 * cosab) / 3.0)**0.5 a_prime = alat / 3**0.5 u = tz - 2 * 2**0.5 * ty v = tz + 2**0.5 * ty cell = np.array([[u, v, v], [v, u, v], [v, v, u]]) * a_prime elif system['ibrav'] == 6: cell = np.array([[1.0, 0.0, 0.0], [0.0, 1.0, 0.0], [0.0, 0.0, c_over_a]]) * alat elif system['ibrav'] == 7: cell = np.array([[1.0, -1.0, c_over_a], [1.0, 1.0, c_over_a], [-1.0, -1.0, c_over_a]]) * (alat / 2) elif system['ibrav'] == 8: cell = np.array([[1.0, 0.0, 0.0], [0.0, b_over_a, 0.0], [0.0, 0.0, c_over_a]]) * alat elif system['ibrav'] == 9: cell = np.array([[1.0 / 2.0, b_over_a / 2.0, 0.0], [-1.0 / 2.0, b_over_a / 2.0, 0.0], [0.0, 0.0, c_over_a]]) * alat elif system['ibrav'] == -9: cell = np.array([[1.0 / 2.0, -b_over_a / 2.0, 0.0], [1.0 / 2.0, b_over_a / 2.0, 0.0], [0.0, 0.0, c_over_a]]) * alat elif system['ibrav'] == 10: cell = np.array([[1.0 / 2.0, 0.0, c_over_a / 2.0], [1.0 / 2.0, b_over_a / 2.0, 0.0], [0.0, b_over_a / 2.0, c_over_a / 2.0]]) * alat elif system['ibrav'] == 11: cell = np.array([[1.0 / 2.0, b_over_a / 2.0, c_over_a / 2.0], [-1.0 / 2.0, b_over_a / 2.0, c_over_a / 2.0], [-1.0, 2.0, -b_over_a / 2.0, c_over_a / 2.0]]) * alat elif system['ibrav'] == 12: sinab = (1.0 - cosab**2)**0.5 cell = np.array([[1.0, 0.0, 0.0], [b_over_a * cosab, b_over_a * sinab, 0.0], [0.0, 0.0, c_over_a]]) * alat elif system['ibrav'] == -12: sinac = (1.0 - cosac**2)**0.5 cell = np.array([[1.0, 0.0, 0.0], [0.0, b_over_a, 0.0], [c_over_a * cosac, 0.0, c_over_a * sinac]]) * alat elif system['ibrav'] == 13: sinab = (1.0 - cosab**2)**0.5 cell = np.array([[1.0 / 2.0, 0.0, -c_over_a / 2.0], [b_over_a * cosab, b_over_a * sinab, 0.0], [1.0 / 2.0, 0.0, c_over_a / 2.0]]) * alat elif system['ibrav'] == 14: sinab = (1.0 - cosab**2)**0.5 v3 = [c_over_a * cosac, c_over_a * (cosbc - cosac * cosab) / sinab, c_over_a * ((1 + 2 * cosbc * cosac * cosab - cosbc**2 - cosac**2 - cosab**2)**0.5) / sinab] cell = np.array([[1.0, 0.0, 0.0], [b_over_a * cosab, b_over_a * sinab, 0.0], v3]) * alat else: raise NotImplementedError('ibrav = {0} is not implemented' ''.format(system['ibrav'])) return alat, cell def get_pseudo_dirs(data): """Guess a list of possible locations for pseudopotential files. Parameters ---------- data : Namelist Namelist representing the quantum espresso input parameters Returns ------- pseudo_dirs : list[str] A list of directories where pseudopotential files could be located. """ pseudo_dirs = [] if 'pseudo_dir' in data['control']: pseudo_dirs.append(data['control']['pseudo_dir']) if 'ESPRESSO_PSEUDO' in os.environ: pseudo_dirs.append(os.environ['ESPRESSO_PSEUDO']) pseudo_dirs.append(path.expanduser('~/espresso/pseudo/')) return pseudo_dirs def get_valence_electrons(symbol, data, pseudo=None): """The number of valence electrons for a atomic symbol. Parameters ---------- symbol : str Chemical symbol data : Namelist Namelist representing the quantum espresso input parameters pseudo : str, optional File defining the pseudopotential to be used. If missing a fallback to the number of valence electrons recommended at http://materialscloud.org/sssp/ is employed. """ if pseudo is None: pseudo = '{}_dummy.UPF'.format(symbol) for pseudo_dir in get_pseudo_dirs(data): if path.exists(path.join(pseudo_dir, pseudo)): valence = grep_valence(path.join(pseudo_dir, pseudo)) break else: # not found in a file valence = SSSP_VALENCE[atomic_numbers[symbol]] return valence def get_atomic_positions(lines, n_atoms, cell=None, alat=None): """Parse atom positions from ATOMIC_POSITIONS card. Parameters ---------- lines : list[str] A list of lines containing the ATOMIC_POSITIONS card. n_atoms : int Expected number of atoms. Only this many lines will be parsed. cell : np.array Unit cell of the crystal. Only used with crystal coordinates. alat : float Lattice parameter for atomic coordinates. Only used for alat case. Returns ------- positions : list[(str, (float, float, float), (float, float, float))] A list of the ordered atomic positions in the format: label, (x, y, z), (if_x, if_y, if_z) Force multipliers are set to None if not present. Raises ------ ValueError Any problems parsing the data result in ValueError """ positions = None # no blanks or comment lines, can the consume n_atoms lines for positions trimmed_lines = (line for line in lines if line.strip() and not line[0] == '#') for line in trimmed_lines: if line.strip().startswith('ATOMIC_POSITIONS'): if positions is not None: raise ValueError('Multiple ATOMIC_POSITIONS specified') # Priority and behaviour tested with QE 5.3 if 'crystal_sg' in line.lower(): raise NotImplementedError('CRYSTAL_SG not implemented') elif 'crystal' in line.lower(): cell = cell elif 'bohr' in line.lower(): cell = np.identity(3) * units['Bohr'] elif 'angstrom' in line.lower(): cell = np.identity(3) # elif 'alat' in line.lower(): # cell = np.identity(3) * alat else: if alat is None: raise ValueError('Set lattice parameter in &SYSTEM for ' 'alat coordinates') # Always the default, will be DEPRECATED as mandatory # in future cell = np.identity(3) * alat positions = [] for _dummy in range(n_atoms): split_line = next(trimmed_lines).split() # These can be fractions and other expressions position = np.dot((infix_float(split_line[1]), infix_float(split_line[2]), infix_float(split_line[3])), cell) if len(split_line) > 4: force_mult = (float(split_line[4]), float(split_line[5]), float(split_line[6])) else: force_mult = None positions.append((split_line[0], position, force_mult)) return positions def get_atomic_species(lines, n_species): """Parse atomic species from ATOMIC_SPECIES card. Parameters ---------- lines : list[str] A list of lines containing the ATOMIC_POSITIONS card. n_species : int Expected number of atom types. Only this many lines will be parsed. Returns ------- species : list[(str, float, str)] Raises ------ ValueError Any problems parsing the data result in ValueError """ species = None # no blanks or comment lines, can the consume n_atoms lines for positions trimmed_lines = (line.strip() for line in lines if line.strip() and not line.startswith('#')) for line in trimmed_lines: if line.startswith('ATOMIC_SPECIES'): if species is not None: raise ValueError('Multiple ATOMIC_SPECIES specified') species = [] for _dummy in range(n_species): label_weight_pseudo = next(trimmed_lines).split() species.append((label_weight_pseudo[0], float(label_weight_pseudo[1]), label_weight_pseudo[2])) return species def get_cell_parameters(lines, alat=None): """Parse unit cell from CELL_PARAMETERS card. Parameters ---------- lines : list[str] A list with lines containing the CELL_PARAMETERS card. alat : float | None Unit of lattice vectors in Angstrom. Only used if the card is given in units of alat. alat must be None if CELL_PARAMETERS card is in Bohr or Angstrom. For output files, alat will be parsed from the card header and used in preference to this value. Returns ------- cell : np.array | None Cell parameters as a 3x3 array in Angstrom. If no cell is found None will be returned instead. cell_alat : float | None If a value for alat is given in the card header, this is also returned, otherwise this will be None. Raises ------ ValueError If CELL_PARAMETERS are given in units of bohr or angstrom and alat is not """ cell = None cell_alat = None # no blanks or comment lines, can take three lines for cell trimmed_lines = (line for line in lines if line.strip() and not line[0] == '#') for line in trimmed_lines: if line.strip().startswith('CELL_PARAMETERS'): if cell is not None: # multiple definitions raise ValueError('CELL_PARAMETERS specified multiple times') # Priority and behaviour tested with QE 5.3 if 'bohr' in line.lower(): if alat is not None: raise ValueError('Lattice parameters given in ' '&SYSTEM celldm/A and CELL_PARAMETERS ' 'bohr') cell_units = units['Bohr'] elif 'angstrom' in line.lower(): if alat is not None: raise ValueError('Lattice parameters given in ' '&SYSTEM celldm/A and CELL_PARAMETERS ' 'angstrom') cell_units = 1.0 elif 'alat' in line.lower(): # Output file has (alat = value) (in Bohrs) if '=' in line: alat = float(line.strip(') \n').split()[-1]) * units['Bohr'] cell_alat = alat elif alat is None: raise ValueError('Lattice parameters must be set in ' '&SYSTEM for alat units') cell_units = alat elif alat is None: # may be DEPRECATED in future cell_units = units['Bohr'] else: # may be DEPRECATED in future cell_units = alat # Grab the parameters; blank lines have been removed cell = [[ffloat(x) for x in next(trimmed_lines).split()[:3]], [ffloat(x) for x in next(trimmed_lines).split()[:3]], [ffloat(x) for x in next(trimmed_lines).split()[:3]]] cell = np.array(cell) * cell_units return cell, cell_alat def str_to_value(string): """Attempt to convert string into int, float (including fortran double), or bool, in that order, otherwise return the string. Valid (case-insensitive) bool values are: '.true.', '.t.', 'true' and 't' (or false equivalents). Parameters ---------- string : str Test to parse for a datatype Returns ------- value : any Parsed string as the most appropriate datatype of int, float, bool or string. """ # Just an integer try: return int(string) except ValueError: pass # Standard float try: return float(string) except ValueError: pass # Fortran double try: return ffloat(string) except ValueError: pass # possible bool, else just the raw string if string.lower() in ('.true.', '.t.', 'true', 't'): return True elif string.lower() in ('.false.', '.f.', 'false', 'f'): return False else: return string.strip("'") def read_fortran_namelist(fileobj): """Takes a fortran-namelist formatted file and returns nested dictionaries of sections and key-value data, followed by a list of lines of text that do not fit the specifications. Behaviour is taken from Quantum ESPRESSO 5.3. Parses fairly convoluted files the same way that QE should, but may not get all the MANDATORY rules and edge cases for very non-standard files: Ignores anything after '!' in a namelist, split pairs on ',' to include multiple key=values on a line, read values on section start and end lines, section terminating character, '/', can appear anywhere on a line. All of these are ignored if the value is in 'quotes'. Parameters ---------- fileobj : file An open file-like object. Returns ------- data : dict of dict Dictionary for each section in the namelist with key = value pairs of data. card_lines : list of str Any lines not used to create the data, assumed to belong to 'cards' in the input file. """ # Espresso requires the correct order data = Namelist() card_lines = [] in_namelist = False section = 'none' # can't be in a section without changing this for line in fileobj: # leading and trailing whitespace never needed line = line.strip() if line.startswith('&'): # inside a namelist section = line.split()[0][1:].lower() # case insensitive if section in data: # Repeated sections are completely ignored. # (Note that repeated keys overwrite within a section) section = "_ignored" data[section] = Namelist() in_namelist = True if not in_namelist and line: # Stripped line is Truthy, so safe to index first character if line[0] not in ('!', '#'): card_lines.append(line) if in_namelist: # parse k, v from line: key = [] value = None in_quotes = False for character in line: if character == ',' and value is not None and not in_quotes: # finished value: data[section][''.join(key).strip()] = str_to_value( ''.join(value).strip()) key = [] value = None elif character == '=' and value is None and not in_quotes: # start writing value value = [] elif character == "'": # only found in value anyway in_quotes = not in_quotes value.append("'") elif character == '!' and not in_quotes: break elif character == '/' and not in_quotes: in_namelist = False break elif value is not None: value.append(character) else: key.append(character) if value is not None: data[section][''.join(key).strip()] = str_to_value( ''.join(value).strip()) return data, card_lines def ffloat(string): """Parse float from fortran compatible float definitions. In fortran exponents can be defined with 'd' or 'q' to symbolise double or quad precision numbers. Double precision numbers are converted to python floats and quad precision values are interpreted as numpy longdouble values (platform specific precision). Parameters ---------- string : str A string containing a number in fortran real format Returns ------- value : float | np.longdouble Parsed value of the string. Raises ------ ValueError Unable to parse a float value. """ if 'q' in string.lower(): return np.longdouble(string.lower().replace('q', 'e')) else: return float(string.lower().replace('d', 'e')) def label_to_symbol(label): """Convert a valid espresso ATOMIC_SPECIES label to a chemical symbol. Parameters ---------- label : str chemical symbol X (1 or 2 characters, case-insensitive) or chemical symbol plus a number or a letter, as in "Xn" (e.g. Fe1) or "X_*" or "X-*" (e.g. C1, C_h; max total length cannot exceed 3 characters). Returns ------- symbol : str The best matching species from ase.utils.chemical_symbols Raises ------ KeyError Couldn't find an appropriate species. Notes ----- It's impossible to tell whether e.g. He is helium or hydrogen labelled 'e'. """ # possibly a two character species # ase Atoms need proper case of chemical symbols. if len(label) >= 2: test_symbol = label[0].upper() + label[1].lower() if test_symbol in chemical_symbols: return test_symbol # finally try with one character test_symbol = label[0].upper() if test_symbol in chemical_symbols: return test_symbol else: raise KeyError('Could not parse species from label {0}.' ''.format(label)) def infix_float(text): """Parse simple infix maths into a float for compatibility with Quantum ESPRESSO ATOMIC_POSITIONS cards. Note: this works with the example, and most simple expressions, but the capabilities of the two parsers are not identical. Will also parse a normal float value properly, but slowly. >>> infix_float('1/2*3^(-1/2)') 0.28867513459481287 Parameters ---------- text : str An arithmetic expression using +, -, *, / and ^, including brackets. Returns ------- value : float Result of the mathematical expression. """ def middle_brackets(full_text): """Extract text from innermost brackets.""" start, end = 0, len(full_text) for (idx, char) in enumerate(full_text): if char == '(': start = idx if char == ')': end = idx + 1 break return full_text[start:end] def eval_no_bracket_expr(full_text): """Calculate value of a mathematical expression, no brackets.""" exprs = [('+', op.add), ('*', op.mul), ('/', op.truediv), ('^', op.pow)] full_text = full_text.lstrip('(').rstrip(')') try: return float(full_text) except ValueError: for symbol, func in exprs: if symbol in full_text: left, right = full_text.split(symbol, 1) # single split return func(eval_no_bracket_expr(left), eval_no_bracket_expr(right)) while '(' in text: middle = middle_brackets(text) text = text.replace(middle, '{}'.format(eval_no_bracket_expr(middle))) return float(eval_no_bracket_expr(text)) ### # Input file writing ### # Ordered and case insensitive KEYS = Namelist(( ('CONTROL', [ 'calculation', 'title', 'verbosity', 'restart_mode', 'wf_collect', 'nstep', 'iprint', 'tstress', 'tprnfor', 'dt', 'outdir', 'wfcdir', 'prefix', 'lkpoint_dir', 'max_seconds', 'etot_conv_thr', 'forc_conv_thr', 'disk_io', 'pseudo_dir', 'tefield', 'dipfield', 'lelfield', 'nberrycyc', 'lorbm', 'lberry', 'gdir', 'nppstr', 'lfcpopt', 'monopole']), ('SYSTEM', [ 'ibrav', 'celldm', 'A', 'B', 'C', 'cosAB', 'cosAC', 'cosBC', 'nat', 'ntyp', 'nbnd', 'tot_charge', 'tot_magnetization', 'starting_magnetization', 'ecutwfc', 'ecutrho', 'ecutfock', 'nr1', 'nr2', 'nr3', 'nr1s', 'nr2s', 'nr3s', 'nosym', 'nosym_evc', 'noinv', 'no_t_rev', 'force_symmorphic', 'use_all_frac', 'occupations', 'one_atom_occupations', 'starting_spin_angle', 'degauss', 'smearing', 'nspin', 'noncolin', 'ecfixed', 'qcutz', 'q2sigma', 'input_dft', 'exx_fraction', 'screening_parameter', 'exxdiv_treatment', 'x_gamma_extrapolation', 'ecutvcut', 'nqx1', 'nqx2', 'nqx3', 'lda_plus_u', 'lda_plus_u_kind', 'Hubbard_U', 'Hubbard_J0', 'Hubbard_alpha', 'Hubbard_beta', 'Hubbard_J', 'starting_ns_eigenvalue', 'U_projection_type', 'edir', 'emaxpos', 'eopreg', 'eamp', 'angle1', 'angle2', 'constrained_magnetization', 'fixed_magnetization', 'lambda', 'report', 'lspinorb', 'assume_isolated', 'esm_bc', 'esm_w', 'esm_efield', 'esm_nfit', 'fcp_mu', 'vdw_corr', 'london', 'london_s6', 'london_c6', 'london_rvdw', 'london_rcut', 'ts_vdw_econv_thr', 'ts_vdw_isolated', 'xdm', 'xdm_a1', 'xdm_a2', 'space_group', 'uniqueb', 'origin_choice', 'rhombohedral', 'zmon', 'realxz', 'block', 'block_1', 'block_2', 'block_height']), ('ELECTRONS', [ 'electron_maxstep', 'scf_must_converge', 'conv_thr', 'adaptive_thr', 'conv_thr_init', 'conv_thr_multi', 'mixing_mode', 'mixing_beta', 'mixing_ndim', 'mixing_fixed_ns', 'diagonalization', 'ortho_para', 'diago_thr_init', 'diago_cg_maxiter', 'diago_david_ndim', 'diago_full_acc', 'efield', 'efield_cart', 'efield_phase', 'startingpot', 'startingwfc', 'tqr']), ('IONS', [ 'ion_dynamics', 'ion_positions', 'pot_extrapolation', 'wfc_extrapolation', 'remove_rigid_rot', 'ion_temperature', 'tempw', 'tolp', 'delta_t', 'nraise', 'refold_pos', 'upscale', 'bfgs_ndim', 'trust_radius_max', 'trust_radius_min', 'trust_radius_ini', 'w_1', 'w_2']), ('CELL', [ 'cell_dynamics', 'press', 'wmass', 'cell_factor', 'press_conv_thr', 'cell_dofree']))) # Number of valence electrons in the pseudopotentials recommended by # http://materialscloud.org/sssp/. These are just used as a fallback for # calculating initial magetization values which are given as a fraction # of valence electrons. SSSP_VALENCE = [ 0, 1.0, 2.0, 3.0, 4.0, 3.0, 4.0, 5.0, 6.0, 7.0, 8.0, 9.0, 10.0, 3.0, 4.0, 5.0, 6.0, 7.0, 8.0, 9.0, 10.0, 11.0, 12.0, 13.0, 14.0, 15.0, 16.0, 17.0, 18.0, 19.0, 20.0, 13.0, 14.0, 5.0, 6.0, 7.0, 8.0, 9.0, 10.0, 11.0, 12.0, 13.0, 14.0, 15.0, 16.0, 17.0, 18.0, 19.0, 12.0, 13.0, 14.0, 15.0, 6.0, 7.0, 18.0, 9.0, 10.0, 11.0, 12.0, 13.0, 14.0, 15.0, 16.0, 17.0, 18.0, 19.0, 20.0, 21.0, 22.0, 23.0, 24.0, 25.0, 36.0, 27.0, 14.0, 15.0, 30.0, 15.0, 32.0, 19.0, 12.0, 13.0, 14.0, 15.0, 16.0, 18.0] def construct_namelist(parameters=None, warn=False, **kwargs): """ Construct an ordered Namelist containing all the parameters given (as a dictionary or kwargs). Keys will be inserted into their appropriate section in the namelist and the dictionary may contain flat and nested structures. Any kwargs that match input keys will be incorporated into their correct section. All matches are case-insensitive, and returned Namelist object is a case-insensitive dict. If a key is not known to ase, but in a section within `parameters`, it will be assumed that it was put there on purpose and included in the output namelist. Anything not in a section will be ignored (set `warn` to True to see ignored keys). Keys with a dimension (e.g. Hubbard_U(1)) will be incorporated as-is so the `i` should be made to match the output. The priority of the keys is: kwargs[key] > parameters[key] > parameters[section][key] Only the highest priority item will be included. Parameters ---------- parameters: dict Flat or nested set of input parameters. warn: bool Enable warnings for unused keys. Returns ------- input_namelist: Namelist pw.x compatible namelist of input parameters. """ # Convert everything to Namelist early to make case-insensitive if parameters is None: parameters = Namelist() else: # Maximum one level of nested dict # Don't modify in place parameters_namelist = Namelist() for key, value in parameters.items(): if isinstance(value, dict): parameters_namelist[key] = Namelist(value) else: parameters_namelist[key] = value parameters = parameters_namelist # Just a dict kwargs = Namelist(kwargs) # Final parameter set input_namelist = Namelist() # Collect for section in KEYS: sec_list = Namelist() for key in KEYS[section]: # Check all three separately and pop them all so that # we can check for missing values later if key in parameters.get(section, {}): sec_list[key] = parameters[section].pop(key) if key in parameters: sec_list[key] = parameters.pop(key) if key in kwargs: sec_list[key] = kwargs.pop(key) # Check if there is a key(i) version (no extra parsing) for arg_key in parameters.get(section, {}): if arg_key.split('(')[0].strip().lower() == key.lower(): sec_list[arg_key] = parameters[section].pop(arg_key) cp_parameters = parameters.copy() for arg_key in cp_parameters: if arg_key.split('(')[0].strip().lower() == key.lower(): sec_list[arg_key] = parameters.pop(arg_key) cp_kwargs = kwargs.copy() for arg_key in cp_kwargs: if arg_key.split('(')[0].strip().lower() == key.lower(): sec_list[arg_key] = kwargs.pop(arg_key) # Add to output input_namelist[section] = sec_list unused_keys = list(kwargs) # pass anything else already in a section for key, value in parameters.items(): if key in KEYS and isinstance(value, dict): input_namelist[key].update(value) elif isinstance(value, dict): unused_keys.extend(list(value)) else: unused_keys.append(key) if warn and unused_keys: warnings.warn('Unused keys: {}'.format(', '.join(unused_keys))) return input_namelist def grep_valence(pseudopotential): """ Given a UPF pseudopotential file, find the number of valence atoms. Parameters ---------- pseudopotential: str Filename of the pseudopotential. Returns ------- valence: float Valence as reported in the pseudopotential. Raises ------ ValueError If valence cannot be found in the pseudopotential. """ # Example lines # Sr.pbe-spn-rrkjus_psl.1.0.0.UPF: z_valence="1.000000000000000E+001" # C.pbe-n-kjpaw_psl.1.0.0.UPF (new ld1.x): # ...PBC" z_valence="4.000000000000e0" total_p... # C_ONCV_PBE-1.0.upf: z_valence=" 4.00" # Ta_pbe_v1.uspp.F.UPF: 13.00000000000 Z valence with open(pseudopotential) as psfile: for line in psfile: if 'z valence' in line.lower(): return float(line.split()[0]) elif 'z_valence' in line.lower(): if line.split()[0] == '<PP_HEADER': line = list(filter(lambda x: 'z_valence' in x, line.split(' ')))[0] return float(line.split('=')[-1].strip().strip('"')) else: raise ValueError('Valence missing in {}'.format(pseudopotential)) def cell_to_ibrav(cell, ibrav): """ Calculate the appropriate `celldm(..)` parameters for the given ibrav using the given cell. The units for `celldm(..)` are Bohr. Does minimal checking of the cell shape, so it is possible to create a nonsense structure if the ibrav is inapproprite for the cell. These are derived to be symmetric with the routine for constructing the cell from ibrav parameters so directions of some vectors may be unexpected. Parameters ---------- cell : np.array A 3x3 representation of a unit cell ibrav : int Bravais-lattice index according to the pw.x designations. Returns ------- parameters : dict A dictionary with all the necessary `celldm(..)` keys assigned necessary values (in units of Bohr). Also includes `ibrav` so it can be passed back to `ibrav_to_cell`. Raises ------ NotImplementedError Only a limited number of ibrav settings can be parsed. An error is raised if the ibrav interpretation is not implemented. """ parameters = {'ibrav': ibrav} if ibrav == 1: parameters['celldm(1)'] = cell[0][0] / units['Bohr'] elif ibrav in [2, 3, -3]: parameters['celldm(1)'] = cell[0][2] * 2 / units['Bohr'] elif ibrav in [4, 6]: parameters['celldm(1)'] = cell[0][0] / units['Bohr'] parameters['celldm(3)'] = cell[2][2] / cell[0][0] elif ibrav in [5, -5]: # Manually derive a = np.linalg.norm(cell[0]) cosab = np.dot(cell[0], cell[1]) / (a ** 2) parameters['celldm(1)'] = a / units['Bohr'] parameters['celldm(4)'] = cosab elif ibrav == 7: parameters['celldm(1)'] = cell[0][0] * 2 / units['Bohr'] parameters['celldm(3)'] = cell[2][2] / cell[0][0] elif ibrav == 8: parameters['celldm(1)'] = cell[0][0] / units['Bohr'] parameters['celldm(2)'] = cell[1][1] / cell[0][0] parameters['celldm(3)'] = cell[2][2] / cell[0][0] elif ibrav in [9, -9]: parameters['celldm(1)'] = cell[0][0] * 2 / units['Bohr'] parameters['celldm(2)'] = cell[1][1] / cell[0][0] parameters['celldm(3)'] = cell[2][2] * 2 / cell[0][0] elif ibrav in [10, 11]: parameters['celldm(1)'] = cell[0][0] * 2 / units['Bohr'] parameters['celldm(2)'] = cell[1][1] / cell[0][0] parameters['celldm(3)'] = cell[2][2] / cell[0][0] elif ibrav == 12: # cos^2 + sin^2 b = (cell[1][0]**2 + cell[1][1]**2)**0.5 parameters['celldm(1)'] = cell[0][0] / units['Bohr'] parameters['celldm(2)'] = b / cell[0][0] parameters['celldm(3)'] = cell[2][2] / cell[0][0] parameters['celldm(4)'] = cell[1][0] / b elif ibrav == -12: # cos^2 + sin^2 c = (cell[2][0]**2 + cell[2][2]**2)**0.5 parameters['celldm(1)'] = cell[0][0] / units['Bohr'] parameters['celldm(2)'] = cell[1][1] / cell[0][0] parameters['celldm(3)'] = c / cell[0][0] parameters['celldm(4)'] = cell[2][0] / c elif ibrav == 13: b = (cell[1][0]**2 + cell[1][1]**2)**0.5 parameters['celldm(1)'] = cell[0][0] * 2 / units['Bohr'] parameters['celldm(2)'] = b / (cell[0][0] * 2) parameters['celldm(3)'] = cell[2][2] / cell[0][0] parameters['celldm(4)'] = cell[1][0] / b elif ibrav == 14: # Manually derive a, b, c = np.linalg.norm(cell, axis=1) cosbc = np.dot(cell[1], cell[2]) / (b * c) cosac = np.dot(cell[0], cell[2]) / (a * c) cosab = np.dot(cell[0], cell[1]) / (a * b) parameters['celldm(1)'] = a / units['Bohr'] parameters['celldm(2)'] = b / a parameters['celldm(3)'] = c / a parameters['celldm(4)'] = cosbc parameters['celldm(5)'] = cosac parameters['celldm(6)'] = cosab else: raise NotImplementedError('ibrav = {0} is not implemented' ''.format(ibrav)) return parameters def kspacing_to_grid(atoms, spacing, calculated_spacing=None): """ Calculate the kpoint mesh that is equivalent to the given spacing in reciprocal space (units Angstrom^-1). The number of kpoints is each dimension is rounded up (compatible with CASTEP). Parameters ---------- atoms: ase.Atoms A structure that can have get_reciprocal_cell called on it. spacing: float Minimum K-Point spacing in $A^{-1}$. calculated_spacing : list If a three item list (or similar mutable sequence) is given the members will be replaced with the actual calculated spacing in $A^{-1}$. Returns ------- kpoint_grid : [int, int, int] MP grid specification to give the required spacing. """ # No factor of 2pi in ase, everything in A^-1 # reciprocal dimensions r_x, r_y, r_z = np.linalg.norm(atoms.cell.reciprocal(), axis=1) kpoint_grid = [int(r_x / spacing) + 1, int(r_y / spacing) + 1, int(r_z / spacing) + 1] for i, _ in enumerate(kpoint_grid): if not atoms.pbc[i]: kpoint_grid[i] = 1 if calculated_spacing is not None: calculated_spacing[:] = [r_x / kpoint_grid[0], r_y / kpoint_grid[1], r_z / kpoint_grid[2]] return kpoint_grid
[docs]def write_espresso_in(fd, atoms, input_data=None, pseudopotentials=None, kspacing=None, kpts=None, koffset=(0, 0, 0), crystal_coordinates=False, **kwargs): """ Create an input file for pw.x. Use set_initial_magnetic_moments to turn on spin, if ispin is set to 2 with no magnetic moments, they will all be set to 0.0. Magnetic moments will be converted to the QE units (fraction of valence electrons) using any pseudopotential files found, or a best guess for the number of valence electrons. Units are not converted for any other input data, so use Quantum ESPRESSO units (Usually Ry or atomic units). Keys with a dimension (e.g. Hubbard_U(1)) will be incorporated as-is so the `i` should be made to match the output. Implemented features: - Conversion of :class:`ase.constraints.FixAtoms` and :class:`ase.constraints.FixCartesian`. - `starting_magnetization` derived from the `mgmoms` and pseudopotentials (searches default paths for pseudo files.) - Automatic assignment of options to their correct sections. - Interpretation of ibrav (cell must exactly match the vectors defined in the QE docs). Not implemented: - Lists of k-points - Other constraints - Hubbard parameters - Validation of the argument types for input - Validation of required options - Reorientation for ibrav settings - Noncollinear magnetism Parameters ---------- fd: file A file like object to write the input file to. atoms: Atoms A single atomistic configuration to write to `fd`. input_data: dict A flat or nested dictionary with input parameters for pw.x pseudopotentials: dict A filename for each atomic species, e.g. {'O': 'O.pbe-rrkjus.UPF', 'H': 'H.pbe-rrkjus.UPF'}. A dummy name will be used if none are given. kspacing: float Generate a grid of k-points with this as the minimum distance, in A^-1 between them in reciprocal space. If set to None, kpts will be used instead. kpts: (int, int, int) or dict If kpts is a tuple (or list) of 3 integers, it is interpreted as the dimensions of a Monkhorst-Pack grid. If ``kpts`` is set to ``None``, only the Γ-point will be included and QE will use routines optimized for Γ-point-only calculations. Compared to Γ-point-only calculations without this optimization (i.e. with ``kpts=(1, 1, 1)``), the memory and CPU requirements are typically reduced by half. If kpts is a dict, it will either be interpreted as a path in the Brillouin zone (*) if it contains the 'path' keyword, otherwise it is converted to a Monkhorst-Pack grid (**). (*) see ase.dft.kpoints.bandpath (**) see ase.calculators.calculator.kpts2sizeandoffsets koffset: (int, int, int) Offset of kpoints in each direction. Must be 0 (no offset) or 1 (half grid offset). Setting to True is equivalent to (1, 1, 1). crystal_coordinates: bool Whether the atomic positions should be written to the QE input file in absolute (False, default) or relative (crystal) coordinates (True). """ # Convert to a namelist to make working with parameters much easier # Note that the name ``input_data`` is chosen to prevent clash with # ``parameters`` in Calculator objects input_parameters = construct_namelist(input_data, **kwargs) # Convert ase constraints to QE constraints # Nx3 array of force multipliers matches what QE uses # Do this early so it is available when constructing the atoms card constraint_mask = np.ones((len(atoms), 3), dtype='int') for constraint in atoms.constraints: if isinstance(constraint, FixAtoms): constraint_mask[constraint.index] = 0 elif isinstance(constraint, FixCartesian): constraint_mask[constraint.a] = constraint.mask else: warnings.warn('Ignored unknown constraint {}'.format(constraint)) # Species info holds the information on the pseudopotential and # associated for each element if pseudopotentials is None: pseudopotentials = {} species_info = {} for species in set(atoms.get_chemical_symbols()): # Look in all possible locations for the pseudos and try to figure # out the number of valence electrons pseudo = pseudopotentials.get(species, None) valence = get_valence_electrons(species, input_parameters, pseudo) species_info[species] = {'pseudo': pseudo, 'valence': valence} # Convert atoms into species. # Each different magnetic moment needs to be a separate type even with # the same pseudopotential (e.g. an up and a down for AFM). # if any magmom are > 0 or nspin == 2 then use species labels. # Rememeber: magnetisation uses 1 based indexes atomic_species = OrderedDict() atomic_species_str = [] atomic_positions_str = [] nspin = input_parameters['system'].get('nspin', 1) # 1 is the default if any(atoms.get_initial_magnetic_moments()): if nspin == 1: # Force spin on input_parameters['system']['nspin'] = 2 nspin = 2 if nspin == 2: # Spin on for atom, magmom in zip(atoms, atoms.get_initial_magnetic_moments()): if (atom.symbol, magmom) not in atomic_species: # spin as fraction of valence fspin = float(magmom) / species_info[atom.symbol]['valence'] # Index in the atomic species list sidx = len(atomic_species) + 1 # Index for that atom type; no index for first one tidx = sum(atom.symbol == x[0] for x in atomic_species) or ' ' atomic_species[(atom.symbol, magmom)] = (sidx, tidx) # Add magnetization to the input file mag_str = 'starting_magnetization({0})'.format(sidx) input_parameters['system'][mag_str] = fspin atomic_species_str.append( '{species}{tidx} {mass} {pseudo}\n'.format( species=atom.symbol, tidx=tidx, mass=atom.mass, pseudo=species_info[atom.symbol]['pseudo'])) # lookup tidx to append to name sidx, tidx = atomic_species[(atom.symbol, magmom)] # only inclued mask if something is fixed if not all(constraint_mask[atom.index]): mask = ' {mask[0]} {mask[1]} {mask[2]}'.format( mask=constraint_mask[atom.index]) else: mask = '' # construct line for atomic positions atomic_positions_str.append( '{atom.symbol}{tidx} ' '{atom.x:.10f} {atom.y:.10f} {atom.z:.10f}' '{mask}\n'.format(atom=atom, tidx=tidx, mask=mask)) else: # Do nothing about magnetisation for atom in atoms: if atom.symbol not in atomic_species: atomic_species[atom.symbol] = True # just a placeholder atomic_species_str.append( '{species} {mass} {pseudo}\n'.format( species=atom.symbol, mass=atom.mass, pseudo=species_info[atom.symbol]['pseudo'])) # only inclued mask if something is fixed if not all(constraint_mask[atom.index]): mask = ' {mask[0]} {mask[1]} {mask[2]}'.format( mask=constraint_mask[atom.index]) else: mask = '' if crystal_coordinates: coords = [atom.a, atom.b, atom.c] else: coords = atom.position atomic_positions_str.append( '{atom.symbol} ' '{coords[0]:.10f} {coords[1]:.10f} {coords[2]:.10f} ' '{mask}\n'.format(atom=atom, coords=coords, mask=mask)) # Add computed parameters # different magnetisms means different types input_parameters['system']['ntyp'] = len(atomic_species) input_parameters['system']['nat'] = len(atoms) # Use cell as given or fit to a specific ibrav if 'ibrav' in input_parameters['system']: ibrav = input_parameters['system']['ibrav'] if ibrav != 0: celldm = cell_to_ibrav(atoms.cell, ibrav) regen_cell = ibrav_to_cell(celldm)[1] if not np.allclose(atoms.cell, regen_cell): warnings.warn('Input cell does not match requested ibrav' '{} != {}'.format(regen_cell, atoms.cell)) input_parameters['system'].update(celldm) else: # Just use standard cell block input_parameters['system']['ibrav'] = 0 # Construct input file into this pwi = [] # Assume sections are ordered (taken care of in namelist construction) # and that repr converts to a QE readable representation (except bools) for section in input_parameters: pwi.append('&{0}\n'.format(section.upper())) for key, value in input_parameters[section].items(): if value is True: pwi.append(' {0:16} = .true.\n'.format(key)) elif value is False: pwi.append(' {0:16} = .false.\n'.format(key)) else: # repr format to get quotes around strings pwi.append(' {0:16} = {1!r:}\n'.format(key, value)) pwi.append('/\n') # terminate section pwi.append('\n') # Pseudopotentials pwi.append('ATOMIC_SPECIES\n') pwi.extend(atomic_species_str) pwi.append('\n') # KPOINTS - add a MP grid as required if kspacing is not None: kgrid = kspacing_to_grid(atoms, kspacing) elif kpts is not None: if isinstance(kpts, dict) and 'path' not in kpts: kgrid, shift = kpts2sizeandoffsets(atoms=atoms, **kpts) koffset = [] for i, x in enumerate(shift): assert x == 0 or abs(x * kgrid[i] - 0.5) < 1e-14 koffset.append(0 if x == 0 else 1) else: kgrid = kpts else: kgrid = "gamma" # True and False work here and will get converted by ':d' format if isinstance(koffset, int): koffset = (koffset, ) * 3 # BandPath object or bandpath-as-dictionary: if isinstance(kgrid, dict) or hasattr(kgrid, 'kpts'): pwi.append('K_POINTS crystal_b\n') assert hasattr(kgrid, 'path') or 'path' in kgrid kgrid = kpts2ndarray(kgrid, atoms=atoms) pwi.append('%s\n' % len(kgrid)) for k in kgrid: pwi.append('{k[0]:.14f} {k[1]:.14f} {k[2]:.14f} 0\n'.format(k=k)) pwi.append('\n') elif isinstance(kgrid, str) and (kgrid == "gamma"): pwi.append('K_POINTS gamma\n') pwi.append('\n') else: pwi.append('K_POINTS automatic\n') pwi.append('{0[0]} {0[1]} {0[2]} {1[0]:d} {1[1]:d} {1[2]:d}\n' ''.format(kgrid, koffset)) pwi.append('\n') # CELL block, if required if input_parameters['SYSTEM']['ibrav'] == 0: pwi.append('CELL_PARAMETERS angstrom\n') pwi.append('{cell[0][0]:.14f} {cell[0][1]:.14f} {cell[0][2]:.14f}\n' '{cell[1][0]:.14f} {cell[1][1]:.14f} {cell[1][2]:.14f}\n' '{cell[2][0]:.14f} {cell[2][1]:.14f} {cell[2][2]:.14f}\n' ''.format(cell=atoms.cell)) pwi.append('\n') # Positions - already constructed, but must appear after namelist if crystal_coordinates: pwi.append('ATOMIC_POSITIONS crystal\n') else: pwi.append('ATOMIC_POSITIONS angstrom\n') pwi.extend(atomic_positions_str) pwi.append('\n') # DONE! fd.write(''.join(pwi))